Asymmetric Brominative Dearomatization of 2-Naphthols Using a Cinchona Alkaloid-Based Organocatalyst

Kouhei Omae,Yoshihiro Miyake,Mio Shimogaki

JOURNAL OF ORGANIC CHEMISTRY（2024）

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摘要

A cinchona alkaloid-based organocatalyst enables asymmetric brominative dearomatization of 2-naphthols, providing the corresponding bromonaphthalenones with high enantioselectivities. The first metal-free reaction can accommodate a variety of functional groups and give useful frameworks bearing a Br-containing tetrasubstituted stereogenic center. [GRAPHICS]

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